A downscaling approach to improve the spatial resolution of Soil Moisture and Ocean Salinity (SMOS) soil moisture estimates with the use of higher resolution visible/infrared (VIS/IR) satellite data is presented. The algorithm is based on the so-called “universal triangle” concept that relates VIS/IR parameters, such as the Normalized Difference Vegetation Index (NDVI), and Land Surface Temperature (Ts), to the soil moisture status. It combines the accuracy of SMOS observations with the high spatial resolution of VIS/IR satellite data into accurate soil moisture estimates at high spatial resolution. In preparation for the SMOS launch, the algorithm was tested using observations of the UPC Airborne RadIomEter at L-band (ARIEL) over the Soil Moisture Measurement Network of the University of Salamanca (REMEDHUS) in Zamora (Spain), and LANDSAT imagery. Results showed fairly good agreement with ground-based soil moisture measurements and illustrated the strength of the link between VIS/IR satellite data and soil moisture status. Following the SMOS launch, a downscaling strategy for the estimation of soil moisture at high resolution from SMOS using MODIS VIS/IR data has been developed. The method has been applied to some of the first SMOS images acquired during the commissioning phase and is validated against in situ soil moisture data from the OZnet soil moisture monitoring network, in South-Eastern Australia. Results show that the soil moisture variability is effectively captured at 10 and 1 km spatial scales without a significant degradation of the root mean square error.